What is it about?
This work demonstrates the feasibility of achieving both high-brightness and high-throughput beam delivery in ultrafast electron microscopy, unlocking unprecedented resolution and sensitivity for multimodal imaging. By leveraging the collective dynamics of high-density photo-emitted electron bunches, the system overcomes traditionally perceived space-charge limitations through the emergence of laminar flow, where stochastic particle trajectories self-organize into a low-momentum, fluid-like state. The case study focuses on observing multiple-order coherent phonon dynamics in 1T-TaSe₂ across timescales ranging from 50 femtoseconds resolution and 10 femtometers sensitivity. This breakthrough showcases the capability of high-brightness electron beams to resolve ultrafast dynamics at atomic scales, enabling precise investigations of complex material behaviors. Key to this achievement is the development of a novel beam control system that operates in the extreme high-density beam regime, overcoming traditional constraints associated with space-charge effects. This innovation paves the way for advanced ultrafast microscopy applications, providing a new platform for exploring material properties with unparalleled spatial, temporal resolutions, and sensitivity.
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Why is it important?
The advancements in high-brightness beam delivery not only redefine the capabilities of ultrafast electron microscopy but also unlock new opportunities in studying phase transitions, catalysis, and quantum materials. By enabling the investigation of nonequilibrium dynamics with femtosecond resolution and nanometer-scale precision, this approach provides a transformative tool for understanding material behaviors under extreme conditions, such as ultrafast switching, energy transport, and structural reconfiguration—phenomena that often remain inaccessible to conventional pump-probe ultrafast electron microscopy operating at high repetition rates.
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This page is a summary of: Precision-controlled ultrafast electron microscope platforms. A case study: Multiple-order coherent phonon dynamics in 1T-TaSe2 probed at 50 fs–10 fm scales, Structural Dynamics, March 2024, American Institute of Physics,
DOI: 10.1063/4.0000242.
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