What is it about?

The investigation on the temporal dynamics of graphene-wrapped core-shell nanoparticles under the illumination of a Gaussian impulse have been carried out. By altering the graphene layers and the aspect ratio of the core-shell structure, we can adjust the resonant modes into typical cases in regime of terahertz. Accordingly, different scenarios for the temporal evolution are detected, which include two kinds of ultrafast oscillation with exponential decay tendency, pure exponential decay, and Gaussian shape, when the pulse duration of the incident pulse is much shorter than, similar to, and much longer than the localized surface plasmon lifetime. To one's interest, when the coupling between two resonant modes exists, one predicts the long-periodic oscillation, whose period is just the difference between the frequencies of the resonant modes. Hence, the intrinsic properties of the ultrafast oscillation can be hardly influenced by the input signals. Further quantitative calculation demonstrate that the periods of the ultrafast oscillations can be tuned by different physical mechanisms, which are respectively based on the self-interacting correction of a single resonance and the strong coupling between the resonant modes in frequency domain. Our results may be applicable in the fields of optical sensors, optical information processing, and other nanophotonic devices.

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Why is it important?

We propose a tunable structure for the modulation on temporal profiles of optical response under the illumination of an ultrashort pulse in the THz range, and reveal the different mechanisms beneath the emergence of ultrafast oscillations in the profiles. With easily tunable physical and geometrical parameters, our structure may offer an applicable method on the operation of ultrafast signals propagation and transferring plasmon framed in optoelectronic nanodevices especially for the length-scale in deep subwavelength.

Perspectives

Writing this article was a great pleasure as it has co-authors with whom I have had long standing collaborations. I hope this article makes people think about the modulation on ultrafast light signal.

Xinchen Jiang
Suzhou City University

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This page is a summary of: Tunable temporal dynamics of dipole response in graphene-wrapped core–shell nanoparticles, Journal of Applied Physics, May 2024, American Institute of Physics,
DOI: 10.1063/5.0208639.
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